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101.
This article presents a simple physical concept of aeolian dust accumulation, based on the behaviour of the subprocesses of dust deposition and dust erosion. The concept is tested in an aeolian dust wind tunnel. The agreement between the accumulation curve predicted by the model and the accumulation curve obtained in the experiments is close to perfect and shows that it is necessary to discriminate between the processes of aeolian dust deposition and aeolian dust accumulation. Two important thresholds determine the accumulation process. For wind speeds below the deflation threshold, the aeolian accumulation of dust increases linearly with the wind speed. For wind velocities between the deflation threshold and the accumulation limit, the sedimentation balance is above unity and there is still accumulation, though it rapidly drops once the deflation threshold has been exceeded. At wind speeds beyond the accumulation limit, the sedimentation balance is below unity and there will no longer be an accumulation of dust. The thresholds have been determined in a wind tunnel test at friction velocity u* = 0·34 m s?1 (deflation threshold) and u* = 0·43 m s?1 (accumulation limit), but these values are only indicative since they depend heavily on the characteristics of the accumulation surface and of the airborne grains. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献   
102.
区域酸性沉降的数值研究 I. 模式   总被引:17,自引:3,他引:17  
王体健  李宗恺  南方 《大气科学》1996,20(5):606-614
建立了一个三维时变的欧拉型区域酸性污染物沉降模式,模式包括源排放、平流输送、湍流扩散、干沉积、气相化学、液相化学及湿清除等六大部分。考虑到计算条件的承受能力和应用性的要求,在把握酸沉降形成的关键过程的前提下,合理地简化设计模式。相对于国内已有的工作,本模式在干沉积、气相化学、液相化学和湿清除等方面均有所改进。  相似文献   
103.
西藏“一江两河”中游地区风成地层沉积时代、沉积相和磁化率等研究结果表明,早在800KaB.P.前西南季风就已存在,受全球气候波动和青藏高原隆起的影响,其盛行衰变与东南季风具有较好的一致性,主要表现为本区地层所记录的气候变化信息不如东南季风区详细;而且西南季风因高原屏障作用给本区带来的降水愈来愈少,气候明显地向干冷化发展。  相似文献   
104.
A small, lightweight (1.5 kg) and fast-response ozone sensor for direct eddy flux measurements has been built. The basis for detection is the chemiluminescence of an organic dye adsorbed on dry silica gel in the reaction with ozone. The chemiluminescence is monitored with a cheap and small blue-sensitive photomultiplier. At a flow rate of 100 l min-1 the ozone sensor has a 90% response time of significantly better than 0.1 s with a detection limit lower than 50 ppt at S/N=3. There are no interferences from other atmospheric trace gases like NOx, H2O2 and PAN. Water vapour and SO2 enhance the chemiluminescence efficiency of the ozone sensor. Since their response times are 22 seconds and 30 minutes, respectively, no correlation between rapid ozone fluctuations and those of these two trace gases is noticed by the ozone sensor when operating at a frequency of 10 Hz.The ozone sensor was tested for several weeks in continuous measurements of ozone fluxes and deposition velocities over different croplands using the eddy correlation technique. Good agreement was found between ozone dry deposition velocities derived from profile measurements and by eddy correlation.  相似文献   
105.
A Eulerian air pollution model for Europe with nonlinear chemistry   总被引:1,自引:0,他引:1  
A long-range transport model with nonlinear chemical reactions is described. The model contains 35 pollutants and 70 chemical reactions. This is a Eulerian model defined on a space domain containing the whole of Europe. The spherical space domain (corresponding to the Earth's surface covered by the model) is mapped into a square plane domain and discretized by using a 32×32 grid. The grid increments are equidistant (both along the Ox axis and along the Oy axis). The choice of values of the physical parameters involved in the model and the numerical treatment of the model are shortly discussed. The model is tested with meteorological data for 1985 and 1989. The numerical results are compared with measurements at stations located in different European countries. Extensive comparisons of ozone concentrations for July 1985 with measurements taken at 24 European stations are also carried out. Results concerning three episodes in July 1985 as well as results obtained in the study of the sensitivity of the ozone concentrations to variations of NO x and/or anthropogenic VOC emissions are presented. The advantages and the limitations of such a model are discussed. The model is continuously improved by adding new modules to it. The plans for improvements in the near future are outlined.  相似文献   
106.
Simultaneous measurements of rain acidity and dimethyl sulfide (DMS) at the ocean surface and in the atmosphere were performed at Amsterdam Island over a 4 year period. During the last 2 years, measurements of sulfur dioxide (SO2) in the atmosphere and of methane sulfonic acid (MSA) and non-sea-salt-sulfate (nss-SO4 2-) in rainwater were also performed. Covariations are observed between the oceanic and atmospheric DMS concentrations, atmospheric SO2 concentrations, wet deposition of MSA, nss-SO4 2-, and rain acidity. A comparable summer to winter ratio of DMS and SO2 in the atmosphere and MSA in precipitation were also observed. From the chemical composition of precipitation we estimate that DMS oxidation products contribute approximately 40% of the rain acidity. If we consider the acidity in excess, then DMS oxidation products contribute about 55%.  相似文献   
107.
黄土中的粘粒含量较高、比表面积较大、吸附性较强、阳离子交换容量也较高,这些因素对迟滞放射性核素的迁移有利。而且黄土的非饱和渗透系数K(θ)远远低于它的饱水渗透系数K_(?)。使得放射性核素在黄土中的迁移很慢。因此,包气带黄土作为中、低放射性废物处置库的环境屏障是可行的。  相似文献   
108.
I. INTRODUCTIONA discharge of 100--200 m3 / s is needed to be diverted from a tidal reach and utilized as cooling water for a Droposed power plant in the Yangtze Estuary. The diversionchannel is divided into two parts by a levee along the river bank, an open channel stretchinside the levee is connected with a trench dredged on the floodplain, as shown in Pig. 1.Since the flow and sediment regimes in these two stretches are different, analysis is madeseparately for each of them.11. ESTI…  相似文献   
109.
The natural distribution of 36Cl/Cl in groundwater across the continental United States has recently been reported by Davis et al. (2003). In this paper, the large-scale processes and atmospheric sources of 36Cl and chloride responsible for controlling the observed 36Cl/Cl distribution are discussed.The dominant process that affects 36Cl/Cl in meteoric groundwater at the continental scale is the fallout of stable chloride from the atmosphere, which is mainly derived from oceanic sources. Atmospheric circulation transports marine chloride to the continental interior, where distance from the coast, topography, and wind patterns define the chloride distribution. The only major deviation from this pattern is observed in northern Utah and southern Idaho where it is inferred that a continental source of chloride exists in the Bonneville Salt Flats, Utah.In contrast to previous studies, the atmospheric flux of 36Cl to the land surface was found to be approximately constant over the United States, without a strong correlation between local 36Cl fallout and annual precipitation. However, the correlation between these variables was significantly improved (R 2=0.15 to R 2=0.55) when data from the southeastern USA, which presumably have lower than average atmospheric 36Cl concentrations, were excluded. The total mean flux of 36Cl over the continental United States and total global mean flux of 36Cl are calculated to be 30.5±7.0 and 19.6±4.5 atoms m–2 s–1, respectively.The 36Cl/Cl distribution calculated by Bentley et al. (1986) underestimates the magnitude and variability observed for the measured 36Cl/Cl distribution across the continental United States. The model proposed by Hainsworth (1994) provides the best overall fit to the observed 36Cl/Cl distribution in this study. A process-oriented model by Phillips (2000) generally overestimates 36Cl/Cl in most parts of the country and has several significant local departures from the empirical data.
Resumen Davis et al. (2003) han informado de la distribución natural de la proporción 36Cl/Cl en las aguas subterráneas de la parte continental de los Estados Unidos de América [EUA]. En este artículo, se discute cuáles son los procesos a gran escala y las fuentes atmosféricas del 36Cl y del cloruro que dan lugar a la distribución observada de 36Cl/Cl.El proceso dominante que afecta a la relación 36Cl/Cl en las aguas subterráneas de origen meteórico a escala continental es el aporte de cloruro estable desde la atmósfera, que procede principalmente de los océanos. La circulación atmosférica transporta el cloruro marino hacia el interior, donde la distancia a la costa, topografía y corrientes del viento definen la distribución del cloruro. La única desviación principal de este esquema tiene lugar al norte de Utah y en el sur de Idaho, donde se deduce que existe una fuente continental de cloruro en los Rellanos Salados de Bonneville (Salt Flats).En contraste con estudios previos (Knies et al. 1994; Phillips 2000), se ha descubierto que el flujo atmosférico de 36Cl hacia la superficie terrestre es aproximadamente constante en todos los estados, sin deducirse una correlación fuerte entre el aporte de 36Cl y la precipitación anual. Sin embargo, la correlación entre estas variables se ve mejorada de forma significativa, con coeficientes de regresión comprendidos entre 0,15 y 0,55, cuando se excluyen los datos recogidos en el sudeste de los EUA, que tienen concentraciones de 36Cl atmosférico presuntamente inferiores a la media. El flujo medio total de 36Cl calculado en la zona continental de los Estados Unidos vale 30,5±7,0 átomos por metro cuadrado y segundo, mientras que el flujo total global de 36Cl es de 19,6±4,5 átomos por metro cuadrado y segundo.La distribución de 36Cl/Cl calculada por Bentley et al. (1986) infravalora la magnitud y variabilidad observada en los valores medidos a lo largo de los Estados Unidos. El modelo propuesto por Hainsworth (1994) proporciona el mejor ajuste conjunto a la distribución observada de 36Cl/Cl en este estudio. El modelo orientado a procesos de Phillips (2000) sobreestima por lo general la distribución de 36Cl/Cl en la mayoría del país y difiere significativamente de algunos valores locales empíricos.

Résumé La distribution naturelle du rapport 36Cl/Cl dans les eaux souterraines des États-Unis a été récemment présentée par Davis et al. (2003). Dans ce travail, les processus à grande échelle et les sources atmosphériques de 36Cl et de chlorure responsables du contrôle de la distribution observée du rapport 36Cl/Cl sont discutés. Le processus dominant qui affecte le rapport 36Cl/Cl dans les eaux souterraines dorigine météorique à léchelle continentale est lapport atmosphérique de chlorure stable, qui provient pour lessentiel de sources océaniques. La circulation atmosphérique transporte des chlorures marins vers lintérieur des continents, où la distribution de chlorure est définie par la distance à la côte, la topographie et les régimes des vents. La seule exception majeure à ce schéma est observée dans le nord de lUtah et le sud de lIdaho où lon suppose quil existe une source continentale de chlorure dans les bas-fonds salés de Bonneville. Au contraire de précédentes études (Knies et al. 1994; Phillips 2000), on trouve que le flux atmosphérique de 36Cl vers le sol est approximativement constant sur lensemble des États-Unis, sans forte corrélation entre la retombée locale de 36Cl et les précipitations annuelles. Cependant, la corrélation entre ces variables devient significative (R 2=0.15 à 0.55) lorsquon supprime les données du sud-est des États-Unis, dont on pense quelles présentent des concentrations en 36Cl atmosphérique inférieures à la moyenne. Le flux total moyen de 36Cl sur les États-Unis continentaux et le flux moyen global de 36Cl sont respectivement évalués à 30.5 ± 7.0 et 19.6 ± 4.5 atomes.m–2.s–1. La distribution du rapport 36Cl/Cl calculée par Bentley et al. (1986) sous-estime lordre de grandeur et la variabilité observés pour la distribution mesurée du rapport 36Cl/Cl sur les États-Unis continentaux. Le modèle proposé par Hainsworth (1994) fournit le meilleur ajustement densemble à la distribution du rapport 36Cl/Cl observée dans cette étude. Un modèle orienté vers les processus proposé par Phillips (2000) surestime dans lensemble le rapport 36Cl/Cl dans la plupart des régions du pays et présente plusieurs désaccords locaux avec les données empiriques.
  相似文献   
110.
The paper presents monitoring results and environmental pollution assessment for the Gdask-Sopot-Gdynia Tricity (Poland), based onanalysis of precipitation. Precipitation samples were collected over a period of 12 months (January–December 1998) at ten locations in the Tricity. The following selected ions were determined in the samples:SO4 2–, F, Cl, NO3 ,PO4 3–, NH4 +, Na+,Mg2+, Ca2+, K+. The results were subjected to full statistical evaluation. Values of the parameters determined were correlated with each other. An attempt was made to explain co-occurrences of certain ions and the significance of their mutual effects. Pollutant concentrations and loads in precipitation were also correlated with data on wind direction and temperature in the region.Deposition of pollutants was very high in spring due to the prevailing air circulation patterns and low temperatures. Analysis of the correlations between co-occurring ions confirmed the significant impact of the location (sea coast) on the composition of rain water. Ionic ratios in rainwater were similar to those observed for sea salt samples. In addition, heavy traffic was most probably responsible for high concentrations of various forms of nitrogen and sulphates in the vicinity of major highways.  相似文献   
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